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The problem of developing scientific foundations for obtaining organic-inorganic materials of a new generation is relevant for solving a number of problems in medicine, chemical industry, engineering, etc. These questions can be solved with the help of new technologies for the synthesis of highly efficient nanostructured catalysts containing various components. Methods for introducing nanostructured components into the composition of the catalytic system are associated with immobilization, sol-gel process, and chemical grafting on the surface of solid materials. In recent years, significant progress has been made in the world in the creation and study of the properties of modified nanostructured heterogeneous catalysts for the vinylation of organic compounds containing active hydrogen atoms. As a result of chemical modification, it was possible to create new, practically important, highly specific selective catalysts, active fillers of polymers, effective thickeners of dispersionmedia.