Iron-Catalysed Hydrofunctionalisation of Alkenes and Alkynes - Greenhalgh, Mark
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Thisthesis gives a thorough account of the development of iron-catalysedhydrosilylation, hydroboration and hydromagnesiation reactions. Withextraordinary referencing and scientific argument, Mark Greenhalgh describesthe development of methodologies which require only commercially availablematerials and non-specialised techniques. The intention of this approach is toensure the science can be adopted widely by the chemical community. In additionto an insight into the processes involved in methodology development, Greenhalghdiscusses and determines the relevant reaction mechanisms. This thesis…mehr

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Produktbeschreibung
Thisthesis gives a thorough account of the development of iron-catalysedhydrosilylation, hydroboration and hydromagnesiation reactions. Withextraordinary referencing and scientific argument, Mark Greenhalgh describesthe development of methodologies which require only commercially availablematerials and non-specialised techniques. The intention of this approach is toensure the science can be adopted widely by the chemical community. In additionto an insight into the processes involved in methodology development, Greenhalghdiscusses and determines the relevant reaction mechanisms. This thesis providesnot only the most thorough review of the area, but offers a level of insightwell beyond that expected from a Ph.D. student. The work in this thesis hasbeen published at the highest level, and the results and ideas have led to 3industry-funded Ph.D. studentships and grant income in excess of £1 million.
Autorenporträt
Mark studied Chemistry with a year in Australia at the University of Sheffield, graduating in 2010 after completing his final year project with Dr Simon Jones. He joined the Chemical Synthesis DTC at the University of Bristol in 2010, and began his PhD the following year with Dr Steve Thomas and Prof. Paul Pringle on iron-catalysed hydrofunctionalisation of alkenes and alkynes. He moved with Steve to the University of Edinburgh in 2012 to complete his PhD studies. Mark has recently moved to St. Andrews to work with Prof. Andrew Smith on the development of Lewis base-catalysed asymmetric methodologies.