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Pyrimidine derivatives, undoubtedly have been of huge interest for the chemists and biologists ascribed to their various properties such as anti-inflammatory, anti-HIV, anti-cancer, anti-malarial and many others. Present book entertains a relative new approach for the synthesis of Pyrimidine derivatives in a much less time, using the modified Biginelli reaction. The derivatives thus synthesized are employed for the their pharmacological activities.